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In the couple of years leading up to her debut album, True Romance, Charli XCX issued a slew of singles, EPs, and mixtapes that mixed moody synth pop with rap and R&B into a sound billed as "neon goth." Despite that somewhat awkward description of her style, Charli does have a flair for chiaroscuro, switching easily from brooding ("Set Me Free") to sparkly ("Take My Hand"), sometimes within the course of one song ("You're the One," one of five previously released tracks here). In some ways, she's the opposite of Grimes, who sprinkles just enough sugar over her quirky musical ideas to make them accessible. Instead, Charli XCX's songs are pop with a capital P – she's unabashed in her love for Britney and Mariah – but just odd enough to be unique. Like Quentin Tarantino, to whom True Romance's title pays homage, she has a flair for combining a wide array of pop culture sources into something fresh and familiar, as well as a fondness for strong female characters.

How I'm Feeling Now is the fourth studio album by English singer and songwriter Charli XCX, released on 15 May 2020. The album was released eight months after her previous album Charli (2019) and was made in a "do-it-yourself" collaborative process with her fans in the span of six weeks. The recording and title were inspired by the COVID-19 pandemic lockdown. Charli XCX, A. G. Cook and BJ Burton served as the album's executive producers. How I'm Feeling Now was preceded by the singles "Forever", "Claws" and "I Finally Understand" which were met with positive reviews from critics. The album received critical acclaim, and was noted for its fusion of pop songwriting and experimental electronic production. It was shortlisted for the 2020 Mercury Prize.

Crash is the fifth studio album by English singer-songwriter Charli XCX, released on 18 March 2022. It is her last album to be released under her current record contract with Atlantic Records. Charli announced the album title, release date, and artwork on 4 November 2021. Her website was also updated with information about the album's 2022 tour. The album was preceded by the four singles "Good Ones", "New Shapes" featuring Christine and the Queens and Caroline Polachek, "Beg for You" featuring Rina Sawayama, "Baby" and two promotional singles, "Every Rule" and "Used to Know Me".

Charli is the third studio album by English singer Charli XCX. It was released through Asylum and Atlantic Records UK on 13 September 2019. Charli XCX's initial third studio album was planned for release in 2017, but was scrapped in its entirety following online leaks. The album will be supported by a world tour, beginning in Atlanta on 20 September 2019. Charli was preceded by the singles "1999" with Troye Sivan, "Blame It on Your Love" featuring Lizzo, and "Gone" with Christine and the Queens. Charli was also promoted by the promotional singles "Cross You Out" featuring Sky Ferreira, "Warm" featuring Haim, "February 2017" featuring Clairo and Yaeji, and "2099" also featuring Sivan. Upon release, the album was met with critical acclaim, with praise centered on the album's innovative production and songwriting.

Crash is the fifth studio album by English singer-songwriter Charli XCX, released on 18 March 2022. It is her last album to be released under her current record contract with Atlantic Records. Charli announced the album title, release date, and artwork on 4 November 2021. Her website was also updated with information about the album's 2022 tour. The album was preceded by the four singles "Good Ones", "New Shapes" featuring Christine and the Queens and Caroline Polachek, "Beg for You" featuring Rina Sawayama, "Baby" and two promotional singles, "Every Rule" and "Used to Know Me". Whereas Charli's prior work was known for its experimental, hyperpop production, Crash features a more conventional dance pop sound. Songs from the album include elements of pop music of the '80s and '90s, and Charli has cited Janet Jackson, among others, as a musical influence for the album. Upon release, the album received generally positive reviews from music critics.